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Scaling laws of shrinkage induced fragmentation phenomena
by Roland Szatmári, Akio Nakahara, So Kitsunezaki, Ferenc Kun
This is not the latest submitted version.
Submission summary
| Authors (as registered SciPost users): | Ferenc Kun |
| Submission information | |
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| Preprint Link: | https://arxiv.org/abs/2503.06177v2 (pdf) |
| Date submitted: | March 25, 2025, 9:28 p.m. |
| Submitted by: | Ferenc Kun |
| Submitted to: | SciPost Physics |
| Ontological classification | |
|---|---|
| Academic field: | Physics |
| Specialties: |
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| Approach: | Computational |
Abstract
We investigate the shrinkage induced breakup of thin layers of heterogeneous materials attached to a substrate, a ubiquitous natural phenomenon with a wide range of potential applications. Focusing on the evolution of the fragment ensemble, we demonstrate that the system has two distinct phases: damage phase, where the layer is cracked, however, a dominant piece persists retaining the structural integrity of the layer, and a fragmentation phase, where the layer disintegrates into numerous small pieces. Based on finite size scaling we show that the transition between the two phases occurs at a critical damage analogous to continuous phase transitions. At the critical point a fully connected crack network emerges whose structure is controlled by the strength of adhesion to the substrate. In the strong adhesion limit, damage arises from random microcrack nucleation, resembling bond percolation, while weak adhesion facilitates stress concentration and the growth of cracks to large extensions. The critical exponents of the damage to fragmentation transition agree to a reasonable accuracy with those of the two-dimensional Ising model. Our findings provide a novel insights into the mechanism of shrinkage-induced cracking revealing generic scaling laws of the phenomenon.
Author indications on fulfilling journal expectations
- Provide a novel and synergetic link between different research areas.
- Open a new pathway in an existing or a new research direction, with clear potential for multi-pronged follow-up work
- Detail a groundbreaking theoretical/experimental/computational discovery
- Present a breakthrough on a previously-identified and long-standing research stumbling block
Current status:
Reports on this Submission
Report #2 by Hans Herrmann (Referee 2) on 2025-7-13 (Invited Report)
- Cite as: Hans Herrmann, Report on arXiv:2503.06177v2, delivered 2025-07-13, doi: 10.21468/SciPost.Report.11564
Report
Since the finite size scaling is performed by changing the system size just by a factor four and the sizes considered are rather small, the data collapse of Figs.7 and 8 is not very powerful. Therefore, I am convinced that the error bars given in Fig.11 for the exponents beta, gamma and nu obtained in Figs.7 and 8 are far too optimistic. The authors should present a more profound error estimation.
The authors claim that the obtained exponents are in the universality class of the 2d Ising model and state “the adhesion strength …. does not affect the universality class of the transition”. But in Fig.11 one can clearly see a strong dependence of gamma and nu on the adhesion strength (if one takes the error bars seriously).
The numerical evidence for the exponents being equal to the ones of the 2d Ising model is very weak, because of the large error bars discussed before, which allows for the numerical exponents to be in fact consistent with several other universality classes. A percolation transition would be expected if the bond breaking would be completely random. The elastic field induces correlations, which when reaching the critical point, become short range. So, percolation exponents seem a reasonable guess. The authors however put forward an argument for the Ising exponents, which is: “The reason of this universality is that cracks always advance through the failure of nearest neighbor cohesive contacts.” This argument is very superficial and applies equally well to percolation, 3 state Potts model, etc. The authors should remove this empty argument and eventually replace it, if they can, by a more convincing argument which should explicitly include the Ising interaction between binary variables.
The authors should define what is a “regularized Voronoi tessellation”.
The authors should add the missing references to the original work in which surface cracking was introduced for the first time as: P. Meakin, Thin Solid Films 151, 165 (1987) or Colina et al Phys. Rev. B 48, 3666 (1993).
Typos: loading -> leading, strength -> strengths (2x)
Recommendation
Ask for major revision
Report #1 by Anonymous (Referee 1) on 2025-7-8 (Invited Report)
- Cite as: Anonymous, Report on arXiv:2503.06177v2, delivered 2025-07-08, doi: 10.21468/SciPost.Report.11528
Strengths
1) Novel theoretical framework: Clear identification of damage vs fragmentation phases with well-characterized critical transition
2) Comprehensive methodology: Systematic parameter study across multiple system sizes with proper statistical sampling
3) Universal scaling laws: Finite size scaling analysis with critical exponents consistent with 2D Ising model
4) Physical insights: Demonstrates how adhesion strength controls stress field heterogeneity and crack patterns
Weaknesses
1) Critical experimental gap: Fails to address Kooij et al.'s highly relevant sugar glass experiments showing exponential fragment distributions under slow thermal fracture vs power-law under impact - directly relevant to their damage/fragmentation transition
2) Limited validation: No direct comparison with experiments beyond citing previous work
3) Universality claims: Insufficient justification for 2D Ising assignment over alternative mechanisms like percolation
4) Model limitations: 2D constraint and simplified adhesion model may not capture realistic 3D behavior
Report
The theoretical approach is sophisticated and the numerical work comprehensive, but the paper suffers from a fundamental disconnect with experimental reality. The most significant oversight is the complete failure to engage with the sugar glass experiments by Kooij et al., which demonstrate exactly the phenomenon being studied theoretically. These experiments show the same material producing different fragment size distributions under different loading conditions - exponential tails for slow fracture versus power-law for impact fracture. This provides direct experimental support for the authors' theoretical predictions about different fragmentation regimes.
The discrete element model itself is well-constructed and captures important physics, particularly the role of adhesion strength in controlling stress field heterogeneity. The identification of two distinct phases separated by a critical transition is a valuable contribution. However, the claim that this transition belongs to the 2D Ising universality class requires stronger theoretical justification. While the critical exponents are "reasonably close" to Ising values, the authors don't adequately explain why this particular fragmentation process should exhibit Ising-like behavior rather than, for example, percolation-type criticality.
The finite size scaling analysis is technically sound and demonstrates continuous phase transition behavior. The transition from power-law fragment distributions in the subcritical regime to log-normal distributions in the supercritical regime is well-documented and physically reasonable, arising from the binary splitting mechanism that dominates post-critical dynamics.
Recommendation
Major Revision Required
This work addresses an important problem with a novel theoretical perspective, but requires significant improvements.
Requested changes
Essential Revisions:
1) Address experimental validation: Thoroughly discuss Kooij et al.'s sugar glass experiments and their connection to the theoretical predictions
2) Strengthen universality arguments: Provide rigorous justification for the 2D Ising classification
3) Improve statistical analysis: Better quantify uncertainties in critical exponents
Additional Improvements:
4) Expand discussion of 3D limitations
5) Include parameter sensitivity analysis
6) Enhance figure quality and statistical presentation
Recommendation
Ask for major revision
