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Emergent Kitaev materials in synthetic Fermi-Hubbard bilayers

by Daniel González-Cuadra, Alejandro Bermudez

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Submission summary

Authors (as registered SciPost users): Daniel González-Cuadra
Submission information
Preprint Link: https://arxiv.org/abs/2504.15755v2  (pdf)
Date accepted: Nov. 5, 2025
Date submitted: Oct. 23, 2025, 11:08 a.m.
Submitted by: Daniel González-Cuadra
Submitted to: SciPost Physics
Ontological classification
Academic field: Physics
Specialties:
  • Atomic, Molecular and Optical Physics - Theory
  • Condensed Matter Physics - Theory
  • Quantum Physics
Approaches: Theoretical, Computational

Abstract

We investigate the emergence of bond-directional spin-spin interactions in a synthetic Fermi-Hubbard bilayer that can be realized with ultracold fermions in Raman optical lattices. The model exploits synthetic dimensions to couple two honeycomb layers, each corresponding to a different hyperfine atomic state, via Raman-assisted tunneling and, moreover, via an inter-layer Hubbard repulsion due to the cold-atom scattering. In the strong-coupling regime at half filling, we derive effective spin Hamiltonians for the kinetic exchange featuring Kitaev, Heisenberg, off-diagonal exchange ($\Gamma$-couplings), as well as tunable Dzyaloshinskii-Moriya interactions. We identify specific configurations that generate both ferromagnetic and antiferromagnetic Kitaev couplings with various perturbations of relevance to Kitaev materials, providing a tunable platform that can explore how quantum spin liquids emerge from itinerant fermion systems. We analyze the Fermi-liquid and Mott-insulating phases, highlighting a correspondence between Dirac and Majorana quasi-particles, with possible phase transitions thereof. In an extreme anisotropic limit, we show that the model reduces to an inter-layer ribbon in a quasi-1D ladder, allowing for a numerical study of the correlated ground state using matrix product states. We find a transition from a symmetry-protected topological insulator to a Kitaev-like regime characterized by nonlocal string order. Our results establish that cold-atom quantum simulators based on Raman optical lattices can be a playground for extended Kitaev models, bridging itinerant fermionic systems and spin-liquid physics.

Author indications on fulfilling journal expectations

  • Provide a novel and synergetic link between different research areas.
  • Open a new pathway in an existing or a new research direction, with clear potential for multi-pronged follow-up work
  • Detail a groundbreaking theoretical/experimental/computational discovery
  • Present a breakthrough on a previously-identified and long-standing research stumbling block

Author comments upon resubmission

We thank both referees for their careful reading of our manuscript and for their positive and constructive comments. We are especially pleased that both referees find our proposal for realizing Kitaev-type physics in cold-atom systems interesting and worthy of publication in SciPost Physics. Below we respond in detail to the specific comments raised by Referee 2.

Response to Referee 2

We thank the referee for the careful reading of our manuscript and for considering that it "provides a novel and synergetic link between different research areas". We have addressed the referee's suggestions and revised the manuscript accordingly, and below we answer the referee's points one by one.

  1. Provide an outline and the summary of the main results in the beginning of the paper. Optionally, shorten the paper and move some of the parts to Appendices.

We thank the Referee for this suggestions. We have written an extended summary of results at the end of the introduction to clarify the main messages for potential readers. On the other hand, we have decided to maintain the current structure of the paper and avoid adding additional appendices.

  1. Improve Introduction (see Weaknesses)

We thank the Referee for pointing out the seeming understated research in the emergence of Kitaev's quantum spin liquid (QSL) phases from strongly-correlated lattice models of fermions. We agree that this might not have been written with sufficient detail and may lead to a wrong impression.

There are some works, like the seminal papers previously cited as [15,52] which discuss how the quantum compass spin models do in fact arise from a fermionic model in a Mott insulating regime. What we referred to with "emergence" is to set the focus of attention on the possible critical properties when connecting these string-coupling QSL to the non-interacting metallic or semi-metal phases. It is this second question which was, to the best of our knowledge, far less explored (likely because even the strong-coupling physics with all Kitaev-material terms is already complex enough and not entirely understood) and motivated our work.

Following the Referee's suggestion, we have clarified these differences, and also performed a more exhaustive search in the literature for works discussing the emergence of Kitaev's QSL from a semi-metal as one increases interactions. We have indeed found the following papers that use various mean-field techniques to address this emergence for a particular set of parameters in our model, those that connect to a Kitaev-Heisenberg model

S. R. Hassan, P. V. Sriluckshmy, S. K. Goyal, R. Shankar,and D. Senechal, Phys. Rev. Lett. 110, 037201 (2013).

L. Liang, Z. Wang, and Y. Yu, , Phys. Rev. B 90, 075119 (2014).

[25] J. P. L. Faye, D. Senechal, and S. R. Hassan, Phys. Rev. B 89, 115130 (2014).

More recent papers have addressed this model using tensor network techniques, in partiular projected entangled pairs, and auxiliary-field quantum Monte Carlo, identifying qualitative differences with respect to the mean-field predictions

Shaojun Dong, Hao Zhang, Chao Wang, Meng Zhang, Yong-Jian Han and Lixin He, Chinese Phys. Lett. 40 126403 (2023).

F Mohammadi, SM Tabatabaei, M Kargarian, A Vaezi, Phys. Rev. B 110, 214425 (2024)x

We have included these references in the text, and added a paragraph to discuss the corresponding findings.

  1. Some of the Figures, e.g. 1-4 are very heavy and do not contain much information. Perhaps simplify the figures.

We thank the Referee for this suggestion. We would like to note that we already spent a considerable amount of time formatting these figures so that they are rich in content and, yet, visually appealing. We would thus prefer to keep them in the current format.

  1. Check spelling.

We checked and corrected spelling mistakes.

List of changes

  1. Added extended summary of results at the end of the introduction.
  2. Added more references in the introduction.
  3. Checked spelling.

Published as SciPost Phys. 19, 130 (2025)

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