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Correlations and linewidth of the atomic beam continuous superradiant laser

by Bruno Laburthe-Tolra, Ziyad Amodjee, Benjamin Pasquiou, Martin Robert-de-Saint-Vincent

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Submission summary

Authors (as registered SciPost users): Benjamin Pasquiou
Submission information
Preprint Link: https://arxiv.org/abs/2210.05464v1  (pdf)
Date submitted: 2022-10-13 10:55
Submitted by: Pasquiou, Benjamin
Submitted to: SciPost Physics Core
Ontological classification
Academic field: Physics
Specialties:
  • Atomic, Molecular and Optical Physics - Theory
  • Quantum Physics
Approach: Theoretical

Abstract

We propose a minimalistic model to account for the main properties of a continuous superradiant laser, in which a beam of atoms crosses the mode of a high-finesse Fabry-Perot cavity, and collectively emits light into the cavity mode. We focus on the case of weak single atom - cavity cooperativity, and highlight the relevant regime where decoherence due to the finite transit time dominates over spontaneous emission. We propose an original approach where the dynamics of atoms entering and leaving the cavity is described by a Hamiltonian process. This allows deriving the main dynamical equations for the superradiant laser, without the need for a stochastic approach. We derive analytical conditions for a sustained emission and show that the ultimate linewidth is set by the fundamental quantum fluctuations of the collective atomic dipole. We calculate steady-state values of the two-body correlators and show that the continuous superradiant regime is tied to the growth of atom-atom correlations, although these correlations only have a small impact on the laser linewidth.

Current status:
Has been resubmitted

Reports on this Submission

Report 1 by Simon Balthasar Jäger on 2022-10-31 (Invited Report)

  • Cite as: Simon Balthasar Jäger, Report on arXiv:2210.05464v1, delivered 2022-10-31, doi: 10.21468/SciPost.Report.6014

Strengths

- Nice introduction

- Comparison of different methods

- Calculation of various properties of the laser

Weaknesses

- Key assumption is unclear

Report

The authors Bruno Laburthe-Tolra et al. study in their work ``Correlations and linewidth of the atomic beam continuous superradiant laser'' various properties of a superradiant laser based on an atomic beam. In their manuscript the authors begin by introducing a Hamiltonian description to determine the dynamics and spectrum of the superradiant burst of an initially inverted atomic ensemble coupled to a single-mode cavity. Using and modifying this Hamiltonian description the authors derive the mean-field dynamics of an atomic beam which traverses and couples to an optical cavity. In their calculation they include the constant ``refreshing'' due to new atoms entering the cavity and also free-space spontaneous emission. With this the authors are able to derive the mean-field dynamics and steady state which is used to determine the lasing regime of this device. In addition the authors also use Monte-Carlo simulations, phase diffusion arguments, and second-order cumulant methods to determine the linewidth of the light field. The cumulant methods are also used to quantify correlation within the atomic ensemble.

In my opinion this is a well written draft which is interesting and timely regarding the various groups working on superradiant lasing with both trapped atoms and atomic beam configurations. The introduction is very didactic and I appreciate the use and comparison of different methods to analyze the physical model. Therefore my opinion is that this manuscript is in general well suited to be published in SciPost Physics Core.

However, before giving my final approval I have a few minor comments and also (some) main question(s) that I believe should be addressed and commented on by the authors.

Minor comments:

(a) On page 2 the authors highlight that they are using a Hamiltonian description without stochastic terms. To my eyes this is basically the mean-field approximation. In addition, while I agree that the collective emission can be cast into a Hamiltonian, I would be surprised if Eq.(20) of the manuscript can be cast into a (hermitian) Hamiltonian. Can the authors comment on this?

(b) I believe it would be helpful to add a few definitions such that there is less space for confusion. For instance on page 2 the authors define the spin operator and I think it would helpful to express them in the excited and ground state projectors and also define $s^x$ and $s^y$. Also, I have not found the definition of Var() and CoVar() [page 21].

(c) On page 4 the authors get two terms for the integral above Eq. (5). The second term (real part) results in the delta function in the long-time limit which is used to obtain the cavity damping rate. The first term would usually result in a frequency shift, however, the authors claim that it vanishes because of the summation over $k$ and since the integrand is odd in $\omega_k$. If I understood it correctly, the latter is the detuning between the cavity resonance and the $k$-mode of the free electromagnetic field $c|k|$. I would argue assuming that this integral vanishes exactly depends on the properties of the spectral density. Nevertheless, even if this integral does not vanish it only renormalizes the cavity resonance. Could the authors comment on that and maybe add a sentence how they can drop this term?

(d) On page 5 the authors write ''In other words, the laser spectrum is at best Fourier limited by the pulse envelope, so that only a sustained or CW laser can ever reach the very narrow linewidths that are necessary for metrological applications.'' I agree that the linewidth in the pulsed regime is $Ng^2/\kappa$ and in the CW mode it is of course much narrower. Still $Ng^2/\kappa$ can also be very narrow if the linewidth of the atomic transition is very narrow. Therefore I think the statement that the pulsed mode is not useful for metrological applications appears to me too strong.

(e) On page 7 the authors write ''We do no expect that the actual mathematical form chosen for $\eta_j(t)$ impacts the result of our analysis.'' In the past, we have performed simulations with different mode functions, velocity distributions, and also stochastic atom insertion and they have sometimes changed the quantitative results such as threshold and intensity. However, the qualitative behavior was in our simulations the same. Maybe the authors could add the word ''qualitatively''.

(f) Equation (20) is equivalent to the mean-field equations for superradiant lasing of a trapped atomic ensemble where the atoms undergo spontaneous emission with rate $\gamma$ and are repumped at rate $\Gamma/N$. Therefore all subsequent mean-field results must be the same as the ones describing a trapped-atom superradiant laser. I think this should be highlighted in the text directly after Eq. (20). In fact the authors write later on page 12 about the lasing threshold: ''A similar condition has been found in the case of a continuously repumped atomic sample [4].'' I would argue these are not similar but the same conditions if one believes that Eq. (20) (which describes the mean-field dynamics of a trapped atomic ensemble) accurately describes the dynamics of an atomic beam.

With this last comment I also come to the main question.

Main question(s):

On page 8 the authors write: ''Furthermore, we also make the following key assumption: $\langle s^-_{j-N} \rangle= \langle S^-\rangle /N$ .'' They further argue: ''We expect this to be valid deep in the superradiant regime when the natural timescale for dynamics $Ng^2/\kappa$ greatly exceeds the transit rate $\Gamma_R$ .'' Also in their Monte-Carlo simulations, I believe, the authors seem to use this when they write ''The disappearance of an atom from the cavity is described by a discrete reduction of the average atomic operators: $S^\epsilon\to(N-1)/N\times S^\epsilon$ after dynamics has taken place.'' on page 14. This assumption is also used in the second order cumulants if I am not mistaken.

I would argue that the value of $\langle s^-_{j-N} \rangle $ depends on the history of the particle inside of the cavity. To highlight this let me propose an example: The highest efficiency of this laser is reached if every atom emits exactly one photon into the cavity. This means that the atom makes a Rabi cycle (with phase $\pi$) from its excited state to its ground state (where it has no more coherence) and consequently $\langle s^-_{j-N} \rangle =0$. Still, the mean collective dipole $\langle S^-\rangle\sim N$ is very large since every atom inside of the cavity (away from the boundaries) carries coherence. In a beam configuration I would argue that there is a mean evolution of the internal atomic state along the cavity waist. For a homogeneoulsy driven and coupled trapped atomic ensemble every atom is in average in the same state (basically no spatial dependence on the mean field level). In a beam configuration, instead, there is a spatiotemporal spin configuration which allows superradiant emission although the mean inversion $\langle S^z\rangle$ is close to zero (see example above). I believe, this cannot happen for a superradiant laser in a trapped atomic ensemble because population inversion is crucial there. For me, this is one big difference between superradiant lasers based on trapped atomic ensembles and atomic beams

My question is now: how can you assume that every atom has relaxed to $\langle s^-_{j-N} \rangle= \langle S^-\rangle /N$?
The authors propose two scenarios on page 8: (A) the atoms reach a steady state shortly after entering the cavity. In this case I ask : what should the relaxation process be? I can imagine at least two: spontaneous emission or additional interactions e.g. collisions. In that case relaxation would require that the typical relaxation time is short compared to the transit time. But this seems to me a very bad regime for the laser operation because one could expect that these processes broaden the laser line or even destroy superradiance. (B) The second scenario which is proposed is that the trajectories of the atoms are very different such that due to ergodicity $\langle s^-_{j-N} \rangle= \langle S^-\rangle /N$ holds. In the lasing (superradiant) regime, I would argue exactly the opposite is true. Every atom follows in average the same trajectory (since the initial condition is fixed: all atoms enter in the excited state) and only beyond mean-field effects add fluctuations around this trajectory. During their flight each atom sees in average the same cavity field and makes the same Rabi oscillation according to the field intensity and phase.

I think that it is crucial that the authors comment on and discuss further their ''key assumption''. In fact, I find this very interesting since it allows them to map the beam configuration onto a trapped atom configuration (at least on the mean-field level).

  • validity: good
  • significance: good
  • originality: good
  • clarity: good
  • formatting: excellent
  • grammar: excellent

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